Few-emitter lasing in single ultra-small nanocavities
Abstract
Lasers are ubiquitous for information storage, processing, communications, sensing, biological research, and medical applications. To decrease their energy and materials usage, a key quest is to miniaturize lasers down to nanocavities. Obtaining the smallest mode volumes demands plasmonic nanocavities, but for these, gain comes from only single or few emitters. Until now, lasing in such devices was unobtainable due to low gain and high cavity losses. Here, we demonstrate a form of “few emitter lasing” in a plasmonic nanocavity approaching the single-molecule emitter regime. The few-emitter lasing transition significantly broadens, and depends on the number of molecules and their individual locations. We show this non-standard few-emitter lasing can be understood by developing a theoretical approach extending previous weak-coupling theories. Our work paves the way for developing nanolaser applications as well as fundamental studies at the limit of few emitters.
Citation
Ojambati , O S , Arnardottir , K B , Lovett , B W , Keeling , J & Baumberg , J J 2024 , ' Few-emitter lasing in single ultra-small nanocavities ' , Nanophotonics . https://doi.org/10.1515/nanoph-2023-0706
Publication
Nanophotonics
Status
Peer reviewed
ISSN
2192-8614Type
Journal article
Description
Funding: We acknowledge support from EPSRC grants EP/G060649/1, EP/L027151/1, EP/G037221/1, EP/T014032/1, EPSRC NanoDTC, and from the European Research Council (ERC) under Horizon 2020 research and innovation programme PICOFORCE (Grant Agreement No. 883703), THOR (Grant Agreement No. 829067) and POSEIDON (Grant Agreement No. 861950). O.S.O acknowledges the support of a Rubicon fellowship from the Netherlands Organisation for Scientific Research.Collections
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