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Dipolar-coupled entangled molecular 4f qubits

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dc.contributor.authorBode, Bela E.
dc.contributor.authorFusco, Edoardo
dc.contributor.authorNixon, Rachel
dc.contributor.authorBuch, Christian
dc.contributor.authorWeihe, Høgni
dc.contributor.authorPiligkos, Stergios
dc.date.accessioned2023-01-26T11:30:17Z
dc.date.available2023-01-26T11:30:17Z
dc.date.issued2023-02-08
dc.identifier282936259
dc.identifier25e9bc3e-2ade-4dea-b56c-26c130956b5d
dc.identifier85147107540
dc.identifier.citationBode , B E , Fusco , E , Nixon , R , Buch , C , Weihe , H & Piligkos , S 2023 , ' Dipolar-coupled entangled molecular 4f qubits ' , Journal of the American Chemical Society , vol. 145 , no. 5 , pp. 2877-2883 . https://doi.org/10.1021/jacs.2c10902en
dc.identifier.issn0002-7863
dc.identifier.otherORCID: /0000-0002-3384-271X/work/127573632
dc.identifier.urihttps://hdl.handle.net/10023/26834
dc.descriptionFunding: S.P. thanks the Novo Nordisk Foundation for research grant NNF20OC0065610. EPR Equipment funding by BBSRC to B. E. B. (17 Alert grant BB/R013780/1) is also gratefully acknowledged.en
dc.description.abstractWe demonstrate by use of continuous wave- and pulse-electron paramagnetic resonance spectroscopy on oriented single crystals of magnetically dilute YbIII ions in Yb0.01Lu0.99(trensal) that molecular entangled two-qubit systems can be constructed by exploiting dipolar interactions between neighboring YbIII centers. Furthermore, we show that the phase memory time and Rabi frequencies of these dipolar-interaction-coupled entangled two-qubit systems are comparable to the ones of the corresponding single qubits.
dc.format.extent7
dc.format.extent4612021
dc.language.isoeng
dc.relation.ispartofJournal of the American Chemical Societyen
dc.subjectQD Chemistryen
dc.subjectDASen
dc.subjectMCCen
dc.subject.lccQDen
dc.titleDipolar-coupled entangled molecular 4f qubitsen
dc.typeJournal articleen
dc.contributor.sponsorBBSRCen
dc.contributor.institutionUniversity of St Andrews. EaSTCHEMen
dc.contributor.institutionUniversity of St Andrews. Biomedical Sciences Research Complexen
dc.contributor.institutionUniversity of St Andrews. Centre of Magnetic Resonanceen
dc.contributor.institutionUniversity of St Andrews. School of Chemistryen
dc.identifier.doi10.1021/jacs.2c10902
dc.description.statusPeer revieweden
dc.identifier.grantnumberBB/R013780/1en


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