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Dipolar-coupled entangled molecular 4f qubits

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Bode_2023_JACS_Dipolar_coupled_CC.pdf (4.398Mb)
Date
25/01/2023
Author
Bode, Bela E.
Fusco, Edoardo
Nixon, Rachel
Buch, Christian
Weihe, Høgni
Piligkos, Stergios
Funder
BBSRC
Grant ID
BB/R013780/1
Keywords
QD Chemistry
DAS
MCP
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Abstract
We demonstrate by use of continuous wave- and pulse-electron paramagnetic resonance spectroscopy on oriented single crystals of magnetically dilute YbIII ions in Yb0.01Lu0.99(trensal) that molecular entangled two-qubit systems can be constructed by exploiting dipolar interactions between neighboring YbIII centers. Furthermore, we show that the phase memory time and Rabi frequencies of these dipolar-interaction-coupled entangled two-qubit systems are comparable to the ones of the corresponding single qubits.
Citation
Bode , B E , Fusco , E , Nixon , R , Buch , C , Weihe , H & Piligkos , S 2023 , ' Dipolar-coupled entangled molecular 4f qubits ' , Journal of the American Chemical Society , vol. Articles ASAP . https://doi.org/10.1021/jacs.2c10902
Publication
Journal of the American Chemical Society
Status
Peer reviewed
DOI
https://doi.org/10.1021/jacs.2c10902
ISSN
0002-7863
Type
Journal article
Rights
Copyright © 2023 The Authors. Published by American Chemical Society. This is an open access article distributed under the terms of the Creative Commons Attribution License, which permits unrestricted use, distribution, and reproduction in any medium, provided the original author and source are credited.
Description
S.P. thanks the Novo Nordisk Foundation for research grant NNF20OC0065610. EPR Equipment funding by BBSRC to B. E. B. (17 Alert grant BB/R013780/1) is also gratefully acknowledged.
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  • University of St Andrews Research
URI
http://hdl.handle.net/10023/26834

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