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dc.contributor.authorDietrich, Christof Peter
dc.contributor.authorSteude, Anja
dc.contributor.authorTropf, Laura Christine
dc.contributor.authorSchubert, Marcel
dc.contributor.authorKronenberg, Nils Michael
dc.contributor.authorOstermann, Kai
dc.contributor.authorHoefling, Sven
dc.contributor.authorGather, Malte Christian
dc.identifier.citationDietrich , C P , Steude , A , Tropf , L C , Schubert , M , Kronenberg , N M , Ostermann , K , Hoefling , S & Gather , M C 2016 , ' An exciton-polariton laser based on biologically produced fluorescent protein ' , Science Advances , vol. 2 , no. 8 , e1600666 , pp. 1-7 .
dc.identifier.otherPURE: 244546146
dc.identifier.otherPURE UUID: cd89c8eb-59ea-4b9d-a2da-750dab18c455
dc.identifier.otherScopus: 84992215390
dc.identifier.otherORCID: /0000-0002-4857-5562/work/47136517
dc.identifier.otherORCID: /0000-0002-8739-4852/work/36937598
dc.identifier.otherWOS: 000383734300026
dc.descriptionWe thank A. Clemens (TU Dresden, Germany) for technical support with protein preparation and C. Murawski (U St Andrews, UK) for support with TDAF deposition. We acknowledge support from the ERC Starting Grant ABLASE (640012), the Scottish Funding Council (via SUPA), the European Union Marie Curie Career Integration Grant (PCIG12-GA-2012-334407), studentship funding through the EPSRC CM-DTC (EP/L015110/1) and the EPSRC Hybrid Polaritonics program grant (EP/M025330/1). S.H. gratefully acknowledges support by the Royal Society and the Wolfson Foundation and M.S. gratefully acknowledges support from a MSCA IF (659213).en
dc.description.abstractUnder adequate conditions, cavity-polaritons form a macroscopic coherent quantum state, known as polariton condensate (PC). Compared to Wannier-Mott polaritons in inorganic semiconductors, the localized Frenkel polaritons in organic emitter materials show weaker interaction with each other but stronger coupling to light, which recently enabled the first realization of a PC at room temperature. However, this required ultrafast optical pumping which limits the applications of organic PCs. Here, we demonstrate room-temperature PCs of cavity-polaritons in simple laminated microcavities filled with the biologically produced enhanced green fluorescent protein (eGFP). The unique molecular structure of eGFP prevents exciton annihilation even at high excitation densities, thus facilitating PCs under conventional nanosecond pumping. Condensation is clearly evidenced by a distinct threshold, an interaction-induced blueshift of the condensate, long-range coherence and the presence of a second threshold at higher excitation density which is associated with the onset of photon lasing.
dc.relation.ispartofScience Advancesen
dc.rights2016 © The Authors, some rights reserved; exclusive licensee American Association for the Advancement of Science. Distributed under a Creative Commons Attribution License 4.0 (CC BY).en
dc.subjectFluorescent proteinen
dc.subjectQC Physicsen
dc.subjectQH301 Biologyen
dc.titleAn exciton-polariton laser based on biologically produced fluorescent proteinen
dc.typeJournal articleen
dc.description.versionPublisher PDFen
dc.contributor.institutionUniversity of St Andrews.School of Physics and Astronomyen
dc.contributor.institutionUniversity of St Andrews.Condensed Matter Physicsen
dc.contributor.institutionUniversity of St Andrews.Biomedical Sciences Research Complexen
dc.description.statusPeer revieweden

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