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dc.contributor.authorIrvine, John Thomas Sirr
dc.contributor.authorNeagu, Dragos
dc.contributor.authorVerbraeken, Maarten Christiaan
dc.contributor.authorChatzchristodoulou, Christodoulous
dc.contributor.authorGraves, Christopher
dc.contributor.authorMogensen, Mogens
dc.date.accessioned2016-07-10T23:31:20Z
dc.date.available2016-07-10T23:31:20Z
dc.date.issued2016-01-11
dc.identifier.citationIrvine , J T S , Neagu , D , Verbraeken , M C , Chatzchristodoulou , C , Graves , C & Mogensen , M 2016 , ' Evolution of the electrochemical interface in high-temperature fuel cells and electrolysers ' , Nature Energy , vol. 1 , 15014 . https://doi.org/10.1038/nenergy.2015.14en
dc.identifier.issn2058-7546
dc.identifier.otherPURE: 240305320
dc.identifier.otherPURE UUID: 422fd40e-0173-490b-a4da-d40d160fb65a
dc.identifier.otherScopus: 85016486351
dc.identifier.otherWOS: 000394094600002
dc.identifier.otherORCID: /0000-0002-8394-3359/work/68280693
dc.identifier.urihttp://hdl.handle.net/10023/9105
dc.descriptionC.C. acknowledges financial support from ECoProbe (DFF – 4005-00129) funded by the Danish Independent Research Council. C.G. and M.B.M. acknowledge financial support from Energinet.dk through the ForskEL programme Solid Oxide Fuel Cells for the Renewable Energy Transition contract no. 2014-1-12231. J.T.S.I., M.C.V. and D.N. acknowledge support from EPSRC Platform Grant EP/K015540/1, EPSRC Tailoring of microstructural evolution in impregnated SOFC electrodes EP/M014304/1 and Royal Society Wolfson Merit Award WRMA 2012/R2.en
dc.description.abstractThe critical region determining the performance and lifetime of solid oxide electrochemical systems is normally at the electrode side of the electrode/electrolyte interface. Typically this electrochemically active region only extends a few micrometres and for best performance involves intricate structures and nanocomposites. Much of the most exciting recent research involves understanding processes occurring at this interface and in developing new means of controlling the structure at this interface on the nanoscale. Here we consider in detail the diverse range of materials architectures that may be involved, describe the evolution of these interface structures and finally explore the new chemistries that allow control and manipulation of these architectures to optimize both performance and durability.
dc.format.extent13
dc.language.isoeng
dc.relation.ispartofNature Energyen
dc.rightsCopyright 2016 the Authors. This work is made available online in accordance with the publisher’s policies. This is the author created, accepted version manuscript following peer review and may differ slightly from the final published version. The final published version of this work is available at: https://dx.doi.org/10.1038/nenergy.2015.14en
dc.subjectQD Chemistryen
dc.subjectE-NDASen
dc.subjectBDCen
dc.subjectR2Cen
dc.subject.lccQDen
dc.titleEvolution of the electrochemical interface in high-temperature fuel cells and electrolysersen
dc.typeJournal articleen
dc.description.versionPostprinten
dc.contributor.institutionUniversity of St Andrews.School of Chemistryen
dc.contributor.institutionUniversity of St Andrews.EaSTCHEMen
dc.identifier.doihttps://doi.org/10.1038/nenergy.2015.14
dc.description.statusPeer revieweden
dc.date.embargoedUntil2016-07-11


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