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dc.contributor.authorUlstrup, Søren
dc.contributor.authorJohannsen, Jens Christian
dc.contributor.authorCilento, Federico
dc.contributor.authorCrepaldi, Alberto
dc.contributor.authorMiwa, Jill A.
dc.contributor.authorZacchigna, Michele
dc.contributor.authorCacho, Cephise
dc.contributor.authorChapman, Richard T.
dc.contributor.authorSpringate, Emma
dc.contributor.authorFromm, Felix
dc.contributor.authorRaidel, Christian
dc.contributor.authorSeyller, Thomas
dc.contributor.authorKing, Phil D.C.
dc.contributor.authorParmigiani, Fulvio
dc.contributor.authorGrioni, Marco
dc.contributor.authorHofmann, Philip
dc.date.accessioned2016-04-22T23:32:41Z
dc.date.available2016-04-22T23:32:41Z
dc.date.issued2015-04
dc.identifier.citationUlstrup , S , Johannsen , J C , Cilento , F , Crepaldi , A , Miwa , J A , Zacchigna , M , Cacho , C , Chapman , R T , Springate , E , Fromm , F , Raidel , C , Seyller , T , King , P D C , Parmigiani , F , Grioni , M & Hofmann , P 2015 , ' Ramifications of optical pumping on the interpretation of time-resolved photoemission experiments on graphene ' , Journal of Electron Spectroscopy and Related Phenomena , vol. 200 , pp. 340–346 . https://doi.org/10.1016/j.elspec.2015.04.010en
dc.identifier.issn0368-2048
dc.identifier.otherPURE: 183308814
dc.identifier.otherPURE UUID: 41171a0a-4756-4297-b6b5-0d82d67ade19
dc.identifier.otherBibtex: urn:bfcbf65756ba76692f158c95dd040285
dc.identifier.otherScopus: 84942297122
dc.identifier.otherWOS: 000362607600030
dc.identifier.urihttp://hdl.handle.net/10023/8670
dc.descriptionThe authors acknowledge financial support from the VILLUM foundation, The Danish Council for Independent Research / Technology and Production Sciences, the Swiss National Science Foundation (NSF), EPSRC, The Royal Society and the Italian Ministry of University and Research (Grants No. FIRBRBAP045JF2 and No. FIRB-RBAP06AWK3). Access to the Artemis Facility was funded by STFC. Work in Chemnitz was supported by the European Union through the project ConceptGraphene, and by the German Research Foundation in the framework of the SPP 1459 Graphene.en
dc.description.abstractAbstract In pump-probe time and angle-resolved photoemission spectroscopy (TR-ARPES) experiments the presence of the pump pulse adds a new level of complexity to the photoemission process in comparison to conventional ARPES. This is evidenced by pump-induced vacuum space-charge effects and surface photovoltages, as well as multiple pump excitations due to internal reflections in the sample-substrate system. These processes can severely affect a correct interpretation of the data by masking the out-of-equilibrium electron dynamics intrinsic to the sample. In this study, we show that such effects indeed influence TR-ARPES data of graphene on a silicon carbide (SiC) substrate. In particular, we find a time- and laser fluence-dependent spectral shift and broadening of the acquired spectra, and unambiguously show the presence of a double pump excitation. The dynamics of these effects is slower than the electron dynamics in the graphene sample, thereby permitting us to deconvolve the signals in the time domain. Our results demonstrate that complex pump-related processes should always be considered in the experimental setup and data analysis.
dc.language.isoeng
dc.relation.ispartofJournal of Electron Spectroscopy and Related Phenomenaen
dc.rightsCopyright © 2015 Published by Elsevier B.V. This is the author’s version of a work that was accepted for publication in Journal of Electron Spectroscopy and Related Phenomena. Changes resulting from the publishing process, such as peer review, editing, corrections, structural formatting, and other quality control mechanisms may not be reflected in this document. Changes may have been made to this work since it was submitted for publication. A definitive version was subsequently published in Journal of Electron Spectroscopy and Related Phenomena, DOI: https://dx.doi.org/10.1016/j.elspec.2015.04.010en
dc.subjectHot Electronsen
dc.subjectGrapheneen
dc.subjectTime- and Angle-Resolved Photoemissionen
dc.subjectSpace Chargeen
dc.subjectQC Physicsen
dc.subjectNDASen
dc.subject.lccQCen
dc.titleRamifications of optical pumping on the interpretation of time-resolved photoemission experiments on grapheneen
dc.typeJournal articleen
dc.description.versionPostprinten
dc.contributor.institutionUniversity of St Andrews.School of Physics and Astronomyen
dc.contributor.institutionUniversity of St Andrews.Condensed Matter Physicsen
dc.identifier.doihttps://doi.org/10.1016/j.elspec.2015.04.010
dc.description.statusPeer revieweden
dc.date.embargoedUntil2016-04-23


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