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Rapid preparation of binary mixtures of sodium carboxylates as anodes in sodium-ion batteries
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dc.contributor.author | Desai, Aamod V. | |
dc.contributor.author | Ettlinger, Romy | |
dc.contributor.author | Seleghini, Heitor Secco | |
dc.contributor.author | Stanzione, Maximillian G | |
dc.contributor.author | Cabañero, Joel | |
dc.contributor.author | Ashbrook, Sharon Elizabeth | |
dc.contributor.author | Morris, Russell | |
dc.contributor.author | Armstrong, A. Robert | |
dc.date.accessioned | 2024-05-08T15:30:08Z | |
dc.date.available | 2024-05-08T15:30:08Z | |
dc.date.issued | 2024-05-28 | |
dc.identifier | 301311518 | |
dc.identifier | 306fa275-7ef2-4df5-8ef0-1467ed053e87 | |
dc.identifier | 85191313971 | |
dc.identifier.citation | Desai , A V , Ettlinger , R , Seleghini , H S , Stanzione , M G , Cabañero , J , Ashbrook , S E , Morris , R & Armstrong , A R 2024 , ' Rapid preparation of binary mixtures of sodium carboxylates as anodes in sodium-ion batteries ' , Journal of Materials Chemistry A , vol. 12 , no. 20 , pp. 12119-12125 . https://doi.org/10.1039/D3TA06928A | en |
dc.identifier.issn | 2050-7488 | |
dc.identifier.other | RIS: urn:2F4FB37659643E60EDD9BFAE7B4E7A8E | |
dc.identifier.other | ORCID: /0000-0001-7219-3428/work/158122934 | |
dc.identifier.other | ORCID: /0000-0002-4538-6782/work/158123311 | |
dc.identifier.other | ORCID: /0000-0001-7809-0315/work/158123426 | |
dc.identifier.other | ORCID: /0000-0003-4026-1515/work/158123456 | |
dc.identifier.other | ORCID: /0000-0003-1937-0936/work/158123495 | |
dc.identifier.uri | https://hdl.handle.net/10023/29840 | |
dc.description | Funding: This work was supported by Faraday Institution (Grant – FIRG018). The authors thank the Engineering and Physical Sciences Research Council (EPSRC) for the Light Element Facility Grant (EP/T019298/1) and Strategic Equipment Resource Grant (EP/R023751/1). R.E. and R.E.M. gratefully acknowledge the financial support by the European Research Council grant ADOR (Advanced Grant 787073). H.S.S. thanks the Allan Handsel Postgraduate Research Scholarship for Chemistry for funding. | en |
dc.description.abstract | Sodium-ion batteries are emerging as a sustainable solution to tackle the growing global energy demands. In this context, organic electrode materials complement such technologies as they are composed of earth-abundant elements. As organic anodes, sodium carboxylates exhibit promising applicability in a wide range of molecules. To harness the advantages of individual systems and to minimise their limitations, in this work, an approach to form binary mixtures of sodium carboxylates using one-pot, microwave-assisted synthesis is presented. The target mixtures were synthesised in 30 min with disodium naphthalene-2,6-dicarboxylate (Na-NDC) as a common constituent in all. Both components in all mixtures were shown to participate in the charge storage and had a considerable effect on the performance characteristics, such as specific capacity and working voltage, in half and full cell formats. This approach opens a new avenue for enabling organic materials to be considered as more competitive candidates in sodium-ion batteries and promote their use in other material classes to overcome their limitations. | |
dc.format.extent | 662198 | |
dc.language.iso | eng | |
dc.relation.ispartof | Journal of Materials Chemistry A | en |
dc.subject | NDAS | en |
dc.title | Rapid preparation of binary mixtures of sodium carboxylates as anodes in sodium-ion batteries | en |
dc.type | Journal article | en |
dc.contributor.sponsor | The Faraday Institution | en |
dc.contributor.sponsor | EPSRC | en |
dc.contributor.sponsor | EPSRC | en |
dc.contributor.sponsor | European Research Council | en |
dc.contributor.institution | University of St Andrews. School of Chemistry | en |
dc.contributor.institution | University of St Andrews. EaSTCHEM | en |
dc.identifier.doi | https://doi.org/10.1039/D3TA06928A | |
dc.description.status | Peer reviewed | en |
dc.identifier.grantnumber | EP/T005602/1 | en |
dc.identifier.grantnumber | EP/T019298/1 | en |
dc.identifier.grantnumber | EP/R023751/1 | en |
dc.identifier.grantnumber | 787073 | en |
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