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dc.contributor.authorNeagu, Dragos
dc.contributor.authorIrvine, John T S
dc.contributor.authorWang, Jiayue
dc.contributor.authorYildiz, Bilge
dc.contributor.authorOpitz, Alexander Karl
dc.contributor.authorFleig, Juergen
dc.contributor.authorWang, Yuhao
dc.contributor.authorLiu, Jiapeng
dc.contributor.authorShen, Longyun
dc.contributor.authorCiucci, Francesco
dc.contributor.authorRosen, Brian A
dc.contributor.authorXiao, Yongchun
dc.contributor.authorXie, Kui
dc.contributor.authorYang, Guangming
dc.contributor.authorShao, Zongping
dc.contributor.authorZhang, Yubo
dc.contributor.authorReinke, Jakob Michael
dc.contributor.authorSchmauss, Travis A.
dc.contributor.authorBarnett, Scott
dc.contributor.authorMaring, Roelf
dc.contributor.authorKyriakou, Vasileios
dc.contributor.authorMushtaq, Usman
dc.contributor.authorTsampas, Mihalis N.
dc.contributor.authorKim, Youdong
dc.contributor.authorO'Hayre, Ryan
dc.contributor.authorCarrillo, Alfonso J.
dc.contributor.authorRuh, Thomas
dc.contributor.authorLindenthal, Lorenz
dc.contributor.authorSchrenk, Florian
dc.contributor.authorRameshan, Christoph
dc.contributor.authorPapaioannou, Evangelos I.
dc.contributor.authorKousi, Kalliopi
dc.contributor.authorMetcalfe, Ian
dc.contributor.authorXu, Xiaoxiang
dc.contributor.authorLiu, Gang
dc.date.accessioned2023-06-28T14:30:08Z
dc.date.available2023-06-28T14:30:08Z
dc.date.issued2023-06-20
dc.identifier.citationNeagu , D , Irvine , J T S , Wang , J , Yildiz , B , Opitz , A K , Fleig , J , Wang , Y , Liu , J , Shen , L , Ciucci , F , Rosen , B A , Xiao , Y , Xie , K , Yang , G , Shao , Z , Zhang , Y , Reinke , J M , Schmauss , T A , Barnett , S , Maring , R , Kyriakou , V , Mushtaq , U , Tsampas , M N , Kim , Y , O'Hayre , R , Carrillo , A J , Ruh , T , Lindenthal , L , Schrenk , F , Rameshan , C , Papaioannou , E I , Kousi , K , Metcalfe , I , Xu , X & Liu , G 2023 , ' Roadmap on exsolution for energy applications ' , Journal of Physics: Energy , vol. 5 , no. 3 , 031501 . https://doi.org/10.1088/2515-7655/acd146en
dc.identifier.issn2515-7655
dc.identifier.otherPURE: 285338297
dc.identifier.otherPURE UUID: 3c1eaef0-f822-4a00-8fba-de36817ff6d1
dc.identifier.otherBibtex: 10.1088/2515-7655/acd146
dc.identifier.otherORCID: /0000-0002-8394-3359/work/137914790
dc.identifier.otherScopus: 85162693764
dc.identifier.urihttps://hdl.handle.net/10023/27828
dc.descriptionFunding: The authors thank the OxEon Corporation for supporting this work. The authors gratefully acknowledge the financial support from the Research Grants Council of Hong Kong (RGC Ref Nos. 16 201 820 and 16 206 019). This work was supported in part by the Project of Hetao Shenzhen-Hong Kong Science and Technology Innovation Cooperation Zone (HZQB-KCZYB-2020083). We acknowledge the National Key Research and Development, Program of China (2017YFA0700102), Natural Science Foundation of China (91 845 202) and Strategic Priority Research Program of Chinese Academy of Sciences (XDB2000000). The authors acknowledge the financial support from the National Key R&D Program of China (2022YFB4004000). The authors gratefully acknowledge financial support from Department of Energy (DOE) Grant # DE-SC0016965, and DOE Grant # DE-FE0031986, which equally supported the authors in writing this review. This work has been carried out within the ViSEP program (733.000.006) funded jointly by the Netherlands Organization for Scientific Research (N.W.O.) and Shell. Research supported as part of the hydrogen in energy and information sciences, an Energy Frontier Research Center funded by the U.S. DOE, Office of Science, Basic Energy Sciences, under Award #DE-SC0023450. In addition, Y K acknowledges funding from the U.S. Army Research Office through Grant No. W911NF-22-1-0273. The project that gave rise to these results received the support of a fellowship from ‘la Caixa’ Foundation (ID 100 010 434). The fellowship code is LCF/BQ/PI20/11760015. This work was funded by the European Research Council (ERC) under the European Union’s Horizon 2020 research and innovation programme, Grant Agreement No. 755744/ERC—Starting Grant TUCAS. The authors acknowledge DESY (Hamburg, Germany), a member of the Helmholtz Association HGF, for the provision of experimental facilities. Parts of this research were carried out at PETRA III, and the authors would like to thank Henrik Jeppesen for assistance in using beamline P02.1. Beamtime was allocated for proposal I-20211526 EC. The author is grateful for the financial support from the UK Catalysis Hub funded by EPSRC Grant reference EP/R027129/1. The authors wish to thank EPSRC for funding via Grant EP/R023921/1, the Henry Royce Institute (EP/X527257/1), the Royal Society of Chemistry (E22-6433572226) and The Royal Society (RGS\R2\222062). ISM acknowledges funding from the Royal Academy of Engineering through a Chair in Emerging Technologies Award entitled “Engineering Chemical Reactor Technologies for a Low-Carbon Energy Future” (Grant CiET1819\2\57). We thank the National Natural Science Foundation of China (Grant Nos. 51972233, 52172225 and 51825204), Natural Science Foundation of Shanghai (Grant No. 19ZR1459200), Science and Technology Commission of Shanghai Municipality (Grant No. 19DZ2271500) and the Fundamental Research Funds for the Central Universities for funding.en
dc.description.abstractOver the last decade, exsolution has emerged as a powerful new method for decorating oxide supports with uniformly dispersed nanoparticles for energy and catalytic applications. Due to their exceptional anchorage, resilience to various degradation mechanisms, as well as numerous ways in which they can be produced, transformed and applied, exsolved nanoparticles have set new standards for nanoparticles in terms of activity, durability and functionality. In conjunction with multifunctional supports such as perovskite oxides, exsolution becomes a powerful platform for the design of advanced energy materials. In the following sections, we review the current status of the exsolution approach, seeking to facilitate transfer of ideas between different fields of application. We also explore future directions of research, particularly noting the multi-scale development required to take the concept forward, from fundamentals through operando studies to pilot scale demonstrations.
dc.format.extent56
dc.language.isoeng
dc.relation.ispartofJournal of Physics: Energyen
dc.rightsCopyright © 2023 Author(s). Published by IOP Publishing Ltd. Original content from this work mayv be used under the terms of the Creative Commons Attribution 4.0 licence. Any further distribution of this work must maintain attribution to the author(s) and the title of thework, journal citation and DOI.en
dc.subjectExsolutionen
dc.subjectEnergyen
dc.subjectOxidesen
dc.subjectCatalysisen
dc.subjectExsolved nanoparticlesen
dc.subjectQD Chemistryen
dc.subjectQC Physicsen
dc.subjectNDASen
dc.subjectMCCen
dc.subject.lccQDen
dc.subject.lccQCen
dc.titleRoadmap on exsolution for energy applicationsen
dc.typeJournal articleen
dc.description.versionPostprinten
dc.description.versionPublisher PDFen
dc.contributor.institutionUniversity of St Andrews. Centre for Energy Ethicsen
dc.contributor.institutionUniversity of St Andrews. Centre for Designer Quantum Materialsen
dc.contributor.institutionUniversity of St Andrews. School of Chemistryen
dc.contributor.institutionUniversity of St Andrews. EaSTCHEMen
dc.identifier.doihttps://doi.org/10.1088/2515-7655/acd146
dc.description.statusPeer revieweden


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