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Dual NHC/photoredox catalytic synthesis of 1,4-diketones using an MR-TADF photocatalyst (DiKTa)
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dc.contributor.author | Prentice, Callum | |
dc.contributor.author | Morrison, James | |
dc.contributor.author | Zysman-Colman, Eli | |
dc.contributor.author | Smith, Andrew D. | |
dc.date.accessioned | 2022-12-02T16:30:13Z | |
dc.date.available | 2022-12-02T16:30:13Z | |
dc.date.issued | 2022-12-21 | |
dc.identifier | 282081576 | |
dc.identifier | 4bb4003e-b7bc-4cb1-b7cf-427d5878a36b | |
dc.identifier | 85142786179 | |
dc.identifier.citation | Prentice , C , Morrison , J , Zysman-Colman , E & Smith , A D 2022 , ' Dual NHC/photoredox catalytic synthesis of 1,4-diketones using an MR-TADF photocatalyst (DiKTa) ' , Chemical Communications , vol. 58 , no. 98 , pp. 13624-13627 . https://doi.org/10.26434/chemrxiv-2022-20dvn , https://doi.org/10.1039/D2CC05705K | en |
dc.identifier.issn | 1359-7345 | |
dc.identifier.other | ORCID: /0000-0002-2104-7313/work/122720336 | |
dc.identifier.other | ORCID: /0000-0001-7183-6022/work/122720451 | |
dc.identifier.uri | https://hdl.handle.net/10023/26533 | |
dc.description | Funding: The authors thank AstraZeneca and the University of St Andrews for funding (Case studentship to C.P.). | en |
dc.description.abstract | The use of the recently reported organic multi-resonant thermally activated delayed fluorescence (MR-TADF) photocatalyst DiKTa allows for the modular synthesis of 1,4-diketones under mild and metal-free conditions. The reaction proceeds via a three-component relay process in the presence of an N-heterocyclic carbene (NHC) organocatalyst. | |
dc.format.extent | 4 | |
dc.format.extent | 1593586 | |
dc.language.iso | eng | |
dc.relation.ispartof | Chemical Communications | en |
dc.subject | QD Chemistry | en |
dc.subject | NDAS | en |
dc.subject | MCC | en |
dc.subject.lcc | QD | en |
dc.title | Dual NHC/photoredox catalytic synthesis of 1,4-diketones using an MR-TADF photocatalyst (DiKTa) | en |
dc.type | Journal article | en |
dc.contributor.institution | University of St Andrews. School of Chemistry | en |
dc.contributor.institution | University of St Andrews. Centre for Energy Ethics | en |
dc.contributor.institution | University of St Andrews. EaSTCHEM | en |
dc.identifier.doi | 10.26434/chemrxiv-2022-20dvn | |
dc.description.status | Peer reviewed | en |
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