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Mode switching dynamics in organic polariton lasing

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PhysRevB.106.195403.pdf (6.922Mb)
Date
15/11/2022
Author
Moilanen, Antti J.
Arnardóttir, Kristín B.
Keeling, Jonathan
Törmä, Päivi
Funder
EPSRC
The Royal Society of Edinburgh
Grant ID
EP/M025330/1
1949
Keywords
QC Physics
TK Electrical engineering. Electronics Nuclear engineering
DAS
MCC
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Abstract
We study the dynamics of multimode polariton lasing in organic microcavities by using a second-order cumulant equation approach. By inspecting the time evolution of the photon mode occupations, we show that if multiple lasing peaks are observed in time-integrated mode occupations, the reason can be either bi-modal lasing or temporal switching between several modes. The former takes place within a narrow range of parameters while the latter occurs more widely. We find that the origin of the temporal switching is different in the weak- and strong-coupling regimes. At weak coupling slope efficiency is the determining factor, while for strong coupling it is changes in the eigenmodes and gain spectrum upon pumping. This difference is revealed by investigating the photoluminescence and momentum-resolved gain spectra. Our results underscore the importance of understanding the time evolution of the populations when characterizing the lasing behaviour of a multimode polariton system, and show how these features differ between weak and strong coupling.
Citation
Moilanen , A J , Arnardóttir , K B , Keeling , J & Törmä , P 2022 , ' Mode switching dynamics in organic polariton lasing ' , Physical Review B , vol. 106 , no. 19 , 195403 . https://doi.org/10.1103/PhysRevB.106.195403
Publication
Physical Review B
Status
Peer reviewed
DOI
https://doi.org/10.1103/PhysRevB.106.195403
ISSN
2469-9950
Type
Journal article
Rights
Copyright © 2022 American Physical Society. This work has been made available online in accordance with publisher policies or with permission. Permission for further reuse of this content should be sought from the publisher or the rights holder. This is the final published version of the work, which was originally published at https://doi.org/10.1103/PhysRevB.106.195403.
Description
Funding: AJM and PT acknowledge support by the Academy of Finland under project numbers 303351, 307419, 327293, 318987 (QuantERA project RouTe), 318937 (PROFI), and 320167 (Flagship Programme, Photonics Research and Innovation (PREIN)), and by Centre for Quantum Engineering (CQE) at Aalto University. AJM acknowledges financial support by the Jenny and Antti Wihuri Foundation and ETH Zurich Postdoctoral Fellowship. KBA and JK acknowledge financial support from EPSRC program “Hybrid Polaritonics” (EP/M025330/1). KBA acknowledges support from The RSE Saltire Research Award.
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  • University of St Andrews Research
URI
http://hdl.handle.net/10023/26312

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