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Preparation and reactivity of biomass-derived dihydro-dioxins

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dc.contributor.authorMontgomery, James
dc.contributor.authorKempf, Karl
dc.contributor.authorMiles-Barrett, Daniel M.
dc.contributor.authorKempf, Oxana
dc.contributor.authorLebl, Tomas
dc.contributor.authorWestwood, Nicholas J.
dc.date.accessioned2019-11-05T00:36:31Z
dc.date.available2019-11-05T00:36:31Z
dc.date.issued2019-01-10
dc.identifier.citationMontgomery , J , Kempf , K , Miles-Barrett , D M , Kempf , O , Lebl , T & Westwood , N J 2019 , ' Preparation and reactivity of biomass-derived dihydro-dioxins ' , CHEMSUSCHEM , vol. 12 , no. 1 , pp. 190-193 . https://doi.org/10.1002/cssc.201802109en
dc.identifier.issn1864-564X
dc.identifier.otherPURE: 255932266
dc.identifier.otherPURE UUID: 8911eabe-3e44-456b-bb05-48e37d31768d
dc.identifier.otherScopus: 85055953533
dc.identifier.otherORCID: /0000-0002-0269-3221/work/48516815
dc.identifier.otherORCID: /0000-0003-0630-0138/work/56424197
dc.identifier.otherWOS: 000456279600013
dc.identifier.urihttps://hdl.handle.net/10023/18843
dc.descriptionThis work was supported by EPSRC PhD studentships EP/1654168 (JRDM) and EP/1518175 (DMMB) and the Industrial Biotechnology Innovation Centre (DMMB).en
dc.description.abstractThe depolymerisation of the biopolymer lignin can give pure aromatic monomers but selective catalytic approaches remain scarce. Here, an approach was re-routed to deliver an unusual phenolic monomer. This monomer’s instability proved challenging but a degradation study identified strategies to overcome this. Heterocycles and a useful synthetic intermediate were prepared. The range of aromatics available from the b-O-4 unit in lignin was extended.
dc.format.extent4
dc.language.isoeng
dc.relation.ispartofCHEMSUSCHEMen
dc.rightsCopyright © 2018 WILEY‐VCH Verlag GmbH & Co. KGaA, Weinheim. This work has been made available online in accordance with the publisher’s policies. This is the author created accepted version manuscript following peer review and as such may differ slightly from the final published version. The final published version of this work is available at: https://doi.org/10.1002/cssc.201802109en
dc.subjectDihydro-dioxinen
dc.subjectHetereocyclesen
dc.subjectRenewable monomersen
dc.subjectDepolymerisationen
dc.subjectLigninen
dc.subjectQD Chemistryen
dc.subjectNDASen
dc.subjectSDG 7 - Affordable and Clean Energyen
dc.subject.lccQDen
dc.titlePreparation and reactivity of biomass-derived dihydro-dioxinsen
dc.typeJournal articleen
dc.description.versionPostprinten
dc.contributor.institutionUniversity of St Andrews. School of Chemistryen
dc.contributor.institutionUniversity of St Andrews. EaSTCHEMen
dc.contributor.institutionUniversity of St Andrews. Biomedical Sciences Research Complexen
dc.identifier.doihttps://doi.org/10.1002/cssc.201802109
dc.description.statusPeer revieweden
dc.date.embargoedUntil2019-11-05


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