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Chlorine-enabled electron doping in solution-synthesized SnSe thermoelectric nanomaterials

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dc.contributor.authorHan, Guang
dc.contributor.authorPopuri, Srinivas R.
dc.contributor.authorGreer, Heather F.
dc.contributor.authorLlin, Lourdes F.
dc.contributor.authorBos, Jan-Willem G.
dc.contributor.authorZhou, Wuzong
dc.contributor.authorPaul, Douglas J.
dc.contributor.authorMénard, Hervé
dc.contributor.authorKnox, Andrew R.
dc.contributor.authorMontecucco, Andrea
dc.contributor.authorSiviter, Jonathan
dc.contributor.authorMan, Elena A.
dc.contributor.authorLi, Wen-guang
dc.contributor.authorPaul, Manosh C.
dc.contributor.authorGao, Min
dc.contributor.authorSweet, Tracy
dc.contributor.authorFreer, Robert
dc.contributor.authorAzough, Feridoon
dc.contributor.authorBaig, Hasan
dc.contributor.authorMallik, Tapas K.
dc.contributor.authorGregory, Duncan H.
dc.date.accessioned2018-02-21T00:33:06Z
dc.date.available2018-02-21T00:33:06Z
dc.date.issued2017-07-05
dc.identifier.citationHan , G , Popuri , S R , Greer , H F , Llin , L F , Bos , J-W G , Zhou , W , Paul , D J , Ménard , H , Knox , A R , Montecucco , A , Siviter , J , Man , E A , Li , W , Paul , M C , Gao , M , Sweet , T , Freer , R , Azough , F , Baig , H , Mallik , T K & Gregory , D H 2017 , ' Chlorine-enabled electron doping in solution-synthesized SnSe thermoelectric nanomaterials ' , Advanced Energy Materials , vol. 7 , no. 13 , 1602328 . https://doi.org/10.1002/aenm.201602328en
dc.identifier.issn1614-6832
dc.identifier.otherPURE: 248866610
dc.identifier.otherPURE UUID: 386634fc-04ea-4a34-a108-dd8f1464af86
dc.identifier.otherWOS: 000404751700004
dc.identifier.otherScopus: 85013377932
dc.identifier.otherORCID: /0000-0001-9752-7076/work/58055091
dc.identifier.otherWOS: 000404751700004
dc.identifier.otherORCID: /0000-0003-3947-2024/work/138327121
dc.identifier.urihttps://hdl.handle.net/10023/12762
dc.descriptionThis work was financially supported by the EPSRC (EP/K022156/1). SRP and JWGB acknowledge the EPSRC for support (EP/N01717X/1). HFG and WZ acknowledge the EPSRC for the Equipment Grant to purchase Titan Themis 200 microscope (EP/L017008/1).en
dc.description.abstractAn aqueous solution method is developed for the facile synthesis of Cl-containing SnSe nanoparticles in 10 g quantities per batch. The particle size and Cl concentration of the nanoparticles can be efficiently tuned as a function of reaction duration. Hot pressing produces n-type Cl-doped SnSe nanostructured compacts with thermoelectric power factors optimized via control of Cl dopant concentration. This approach, combining an energy-efficient solution synthesis with hot pressing, provides a simple, rapid, and low-cost route to high performance n-type SnSe thermoelectric materials.
dc.format.extent7
dc.language.isoeng
dc.relation.ispartofAdvanced Energy Materialsen
dc.rights© 2017 WILEY-VCH Verlag GmbH & Co. KGaA, Weinheim. This work has been made available online in accordance with the publisher’s policies. This is the author created, accepted version manuscript following peer review and may differ slightly from the final published version. The final published version of this work is available at https://doi.org/10.1002/aenm.201602328en
dc.subjectTin selenideen
dc.subjectSynthesisen
dc.subjectn-typeen
dc.subjectThermoelectricsen
dc.subjectNanomaterialsen
dc.subjectQD Chemistryen
dc.subjectNDASen
dc.subject.lccQDen
dc.titleChlorine-enabled electron doping in solution-synthesized SnSe thermoelectric nanomaterialsen
dc.typeJournal articleen
dc.contributor.sponsorEPSRCen
dc.contributor.sponsorEPSRCen
dc.description.versionPostprinten
dc.contributor.institutionUniversity of St Andrews. EaSTCHEMen
dc.contributor.institutionUniversity of St Andrews. School of Chemistryen
dc.identifier.doihttps://doi.org/10.1002/aenm.201602328
dc.description.statusPeer revieweden
dc.date.embargoedUntil2018-02-20
dc.identifier.urlhttp://onlinelibrary.wiley.com/doi/10.1002/aenm.201602328/full#footer-support-infoen
dc.identifier.grantnumberep/l017008/1en
dc.identifier.grantnumberEP/K031252/1en


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