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Chlorine-enabled electron doping in solution-synthesized SnSe thermoelectric nanomaterials

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dc.contributor.authorHan, Guang
dc.contributor.authorPopuri, Srinivas R.
dc.contributor.authorGreer, Heather F.
dc.contributor.authorLlin, Lourdes F.
dc.contributor.authorBos, Jan-Willem G.
dc.contributor.authorZhou, Wuzong
dc.contributor.authorPaul, Douglas J.
dc.contributor.authorMénard, Hervé
dc.contributor.authorKnox, Andrew R.
dc.contributor.authorMontecucco, Andrea
dc.contributor.authorSiviter, Jonathan
dc.contributor.authorMan, Elena A.
dc.contributor.authorLi, Wen-guang
dc.contributor.authorPaul, Manosh C.
dc.contributor.authorGao, Min
dc.contributor.authorSweet, Tracy
dc.contributor.authorFreer, Robert
dc.contributor.authorAzough, Feridoon
dc.contributor.authorBaig, Hasan
dc.contributor.authorMallik, Tapas K.
dc.contributor.authorGregory, Duncan H.
dc.date.accessioned2018-02-21T00:33:06Z
dc.date.available2018-02-21T00:33:06Z
dc.date.issued2017-07-05
dc.identifier248866610
dc.identifier386634fc-04ea-4a34-a108-dd8f1464af86
dc.identifier000404751700004
dc.identifier85013377932
dc.identifier000404751700004
dc.identifier.citationHan , G , Popuri , S R , Greer , H F , Llin , L F , Bos , J-W G , Zhou , W , Paul , D J , Ménard , H , Knox , A R , Montecucco , A , Siviter , J , Man , E A , Li , W , Paul , M C , Gao , M , Sweet , T , Freer , R , Azough , F , Baig , H , Mallik , T K & Gregory , D H 2017 , ' Chlorine-enabled electron doping in solution-synthesized SnSe thermoelectric nanomaterials ' , Advanced Energy Materials , vol. 7 , no. 13 , 1602328 . https://doi.org/10.1002/aenm.201602328en
dc.identifier.issn1614-6832
dc.identifier.otherORCID: /0000-0001-9752-7076/work/58055091
dc.identifier.otherORCID: /0000-0003-3947-2024/work/138327121
dc.identifier.urihttps://hdl.handle.net/10023/12762
dc.descriptionThis work was financially supported by the EPSRC (EP/K022156/1). SRP and JWGB acknowledge the EPSRC for support (EP/N01717X/1). HFG and WZ acknowledge the EPSRC for the Equipment Grant to purchase Titan Themis 200 microscope (EP/L017008/1).en
dc.description.abstractAn aqueous solution method is developed for the facile synthesis of Cl-containing SnSe nanoparticles in 10 g quantities per batch. The particle size and Cl concentration of the nanoparticles can be efficiently tuned as a function of reaction duration. Hot pressing produces n-type Cl-doped SnSe nanostructured compacts with thermoelectric power factors optimized via control of Cl dopant concentration. This approach, combining an energy-efficient solution synthesis with hot pressing, provides a simple, rapid, and low-cost route to high performance n-type SnSe thermoelectric materials.
dc.format.extent7
dc.format.extent4451841
dc.language.isoeng
dc.relation.ispartofAdvanced Energy Materialsen
dc.subjectTin selenideen
dc.subjectSynthesisen
dc.subjectn-typeen
dc.subjectThermoelectricsen
dc.subjectNanomaterialsen
dc.subjectQD Chemistryen
dc.subjectNDASen
dc.subject.lccQDen
dc.titleChlorine-enabled electron doping in solution-synthesized SnSe thermoelectric nanomaterialsen
dc.typeJournal articleen
dc.contributor.sponsorEPSRCen
dc.contributor.sponsorEPSRCen
dc.contributor.institutionUniversity of St Andrews. EaSTCHEMen
dc.contributor.institutionUniversity of St Andrews. School of Chemistryen
dc.identifier.doi10.1002/aenm.201602328
dc.description.statusPeer revieweden
dc.date.embargoedUntil2018-02-20
dc.identifier.urlhttp://onlinelibrary.wiley.com/doi/10.1002/aenm.201602328/full#footer-support-infoen
dc.identifier.grantnumberep/l017008/1en
dc.identifier.grantnumberEP/K031252/1en


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