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Expansion of the ADOR strategy for the synthesis of new zeolites : the synthesis of IPC-12 from zeolite UOV

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Date
03/04/2017
Author
Kasneryk, Valeryia
Shamzhy, Mariya
Opanasenko, Maksym
Wheatley, Paul S.
Morris, Samuel A.
Russell, Samantha E.
Mayoral, Alvaro
Trachta, Michal
Čejka, Jiří
Morris, Russell E.
Funder
EPSRC
EPSRC
EPSRC
Grant ID
EP/K025112/1
EP/K005499/1
EP/L016419/1
Keywords
ADOR
Germanosilicates
Isoreticular materials
Structure rearrangement
Zeolites
QD Chemistry
DAS
BDC
R2C
Metadata
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Abstract
The assembly-disassembly-organization-reassembly (ADOR) process has been used to disassemble a parent zeolite with the UOV structure type and then reassemble the resulting layers into a novel structure, IPC-12. The structure of the material has previously been predicted computationally and confirmed in our experiments using X-ray diffraction and atomic resolution STEM-HAADF electron microscopy. This is the first successful application of the ADOR process to a material with porous layers.
Citation
Kasneryk , V , Shamzhy , M , Opanasenko , M , Wheatley , P S , Morris , S A , Russell , S E , Mayoral , A , Trachta , M , Čejka , J & Morris , R E 2017 , ' Expansion of the ADOR strategy for the synthesis of new zeolites : the synthesis of IPC-12 from zeolite UOV ' , Angewandte Chemie , vol. 56 , no. 15 , pp. 4324-4327 . https://doi.org/10.1002/anie.201700590
Publication
Angewandte Chemie
Status
Peer reviewed
DOI
https://doi.org/10.1002/anie.201700590
ISSN
0044-8249
Type
Journal article
Rights
Copyright 2017 The Authors. Published by Wiley-VCH Verlag GmbH & Co. KGaA. This is an open access article under the terms of the Creative Commons Attribution License, which permits use, distribution and reproduction in any medium, provided the original work is properly cited.
Description
R.E.M. thanks the Royal Society and the Engineering and Physical Sciences Research Council (Grants EP/K025112/1, EP/K005499/1, EP/L016419/1) for funding work in this area and for providing a Ph.D. studentship to S.E.R. through the Criticat Centre for Doctoral training. R.E.M. and M. O. acknowledge the OP VVV "Excellent Research Teams", project No. CZ.02.1.01/0.0/0.0/15_003/0000417 - CUCAM. J.Č., V.K., and M.T. acknowledge the Czech Science Foundation for the project of the Centre of Excellence (P106/12/G015) and J.Č has received funding from the European Union's Horizon2020 research and innovation programme under grant agreement No 640979. The research leading to these results has received funding from the European Union Seventh Framework Programme under Grant Agreement No. 312483—ESTEEM2 (Integrated Infrastructure Initiative–I3).
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  • University of St Andrews Research
URI
http://hdl.handle.net/10023/10514

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