Expansion of the ADOR strategy for the synthesis of new zeolites : the synthesis of IPC-12 from zeolite UOV
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The assembly-disassembly-organisation-reassembly (ADOR) process has been used to disassemble a parent zeolite with the UOV structure type and then reassemble the resulting layers into a novel structure, IPC-12. The structure of the material has previously been predicted computationally and confirmed in our experiments using X-ray diffraction and atomic resolution STEM-HAADF electron microscopy. This is the first successful application of the ADOR process to a material with porous layers.
Kasneryk , V , Shamzhy , M , Opanasenko , M , Wheatley , P S , Morris , S A , Russell , S E , Mayoral , A , Trachta , M , Čejka , J & Morris , R E 2017 , ' Expansion of the ADOR strategy for the synthesis of new zeolites : the synthesis of IPC-12 from zeolite UOV ' Angewandte Chemie , vol 56 , no. 15 , pp. 4324-4327 . DOI: 10.1002/anie.201700590
Copyright 2017 The Authors. Published by Wiley-VCH Verlag GmbH & Co. KGaA. This is an open access article under the terms of the Creative Commons Attribution License, which permits use, distribution and reproduction in any medium, provided the original work is properly cited.
R.E.M. thanks the Royal Society and the Engineering and Physical Sciences Research Council (Grants EP/K025112/1, EP/K005499/1, EP/L016419/1) for funding work in this area and for providing a Ph.D. studentship to S.E.R. through the Criticat Centre for Doctoral training. R.E.M. and M. O. acknowledge the OP VVV "Excellent Research Teams", project No. CZ.02.1.01/0.0/0.0/15_003/0000417 - CUCAM. J.Č., V.K., and M.T. acknowledge the Czech Science Foundation for the project of the Centre of Excellence (P106/12/G015) and J.Č has received funding from the European Union's Horizon2020 research and innovation programme under grant agreement No 640979. The research leading to these results has received funding from the European Union Seventh Framework Programme under Grant Agreement No. 312483—ESTEEM2 (Integrated Infrastructure Initiative–I3).
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